For some reason, I was thinking along those lines...
Assuming 40 bar for a dive from a 3L (wikipedia says ~1.6 L O2/min, times about 60min), and a minimum of 100 to go in, starting with 60 in the 3, an Ali 80 at 200 should give you 9 dives.
Then you got about 60 in your 3, and a bit more than 100 in your 80, back where you started.
Because of the 100 minimum, cascading from two 80s doesn't give you much, maybe 2/3 extra dives.
I think.
Cheers,
Matthieu